Journal
APPLIED PHYSICS LETTERS
Volume 94, Issue 11, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.3098358
Keywords
energy gap; graphene; photoluminescence; reduction (chemical)
Categories
Funding
- NSF MRSEC [DMR05-20020]
- JSTO DTRA
- ARO [W911NF-06-1-0462]
- DOE [DE-FG02-ER45118]
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We report broadband visible photoluminescence from solid graphene oxide, and modifications of the emission spectrum by progressive chemical reduction. The data suggest a gapping of the two-dimensional electronic system by removal of pi-electrons. We discuss possible gapping mechanisms, and propose that a Kekule pattern of bond distortions may account for the observed behavior.
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