Journal
APPLIED PHYSICS LETTERS
Volume 95, Issue 4, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.3193661
Keywords
adhesion; calcination; electrochemical electrodes; electrospinning; II-VI semiconductors; nanofabrication; nanofibres; solar cells; tensile strength; zinc compounds
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Funding
- A-Star of Singapore [R-279-000-221-305]
- NUS
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A facile method to prepare nanofibrous ZnO photoelectrodes with tunable thicknesses by electrospinning is reported. A self-relaxation layer is formed spontaneously between ZnO nanofibers and fluorine-doped SnO2 (FTO) substrate, which facilitates the release of interfacial tensile stress during calcination, resulting in good adhesion of ZnO film to FTO substrate. Dye-sensitized solar cells (DSSCs) based on the nanofibrous ZnO photoelectrodes are fabricated and an energy conversion efficiency of 3.02% is achieved under irradiation of AM 1.5 simulated sunlight with a power density of 100 mW cm(-2), which shows good promise of electrospun nanofibrous ZnO as the photoelectrode in DSSCs.
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