4.6 Article

Frequency upconverted lasing of nanocrystal quantum dots in microbeads

Journal

APPLIED PHYSICS LETTERS
Volume 95, Issue 18, Pages -

Publisher

AMER INST PHYSICS
DOI: 10.1063/1.3242352

Keywords

biexcitons; microcavities; micromechanical resonators; nanostructured materials; optical pumping; photoluminescence; radiative lifetimes; semiconductor quantum dots; silicon compounds; stimulated emission; time resolved spectra; two-photon processes; whispering gallery modes

Funding

  1. National Science Foundation [ECCS-0824186, ECCS-0846818, 0638209]
  2. Army Research Office [DAAD19-02-D-0001, DURIP 2008-02136]
  3. Directorate For Engineering
  4. Div Of Industrial Innovation & Partnersh [0638209] Funding Source: National Science Foundation
  5. Div Of Electrical, Commun & Cyber Sys
  6. Directorate For Engineering [0846818, 0824186] Funding Source: National Science Foundation

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Stable, frequency upconverted lasing of semiconductor nanocrystal quantum dots was demonstrated in silica microbeads under two-photon pumping conditions. Upon infrared excitation, the stimulated emission of the nanocrystal-doped microbeads exhibits sharp peaks at lambda similar to 610 nm with narrow line widths of < 1 nm. The lasing action has been attributed to the biexciton gain coupled to the whispering gallery modes in spherical cavities, as confirmed by time-resolved photoluminescence spectra. The lasing lifetime characterized in term of pulse numbers (similar to 10(6) pulses) was two orders of magnitude longer than that of the dye salt-based two-photon lasers.

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