4.6 Article

Unambiguous evidence for magnetoelectric coupling of multiferroic origin in 0.73BiFeO3-0.27PbTiO3

Journal

APPLIED PHYSICS LETTERS
Volume 94, Issue 1, Pages -

Publisher

AMER INST PHYSICS
DOI: 10.1063/1.3068000

Keywords

antiferromagnetic materials; bismuth compounds; ferroelectric materials; ferroelectric transitions; lattice constants; lead compounds; magnetisation; magnetoelectric effects; multiferroics; Neel temperature; permittivity; space charge

Funding

  1. Senior Research Fellowship of CSIR, India

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Magnetization, frequency dependent dielectric, and structural studies on 0.73BiFeO(3)-0.27PbTiO(3) in the temperature range from 300 to 600 K reveal anomalies in the unit cell parameters and the intrinsic value of the dielectric constant, free from space charge contributions, at the antiferromagnetic transition temperature (T-N). Our results provide unambiguous confirmation of magnetoelectric coupling of multiferroic origin at T-N and evidence for monoclinic distortion of the ferroelectric phase.

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