Journal
CHEMICAL PHYSICS LETTERS
Volume 399, Issue 4-6, Pages 349-353Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.cplett.2004.10.015
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We report a rational synthetic approach for the preparation of the negatively charged water tetramer anion, the only member of the homogeneous (H2O)(n)(-) series that has been curiously 'missing' in previous reports of these cluster anions. The synthesis was carried out using argon cluster-mediated anion formation. The identity of the (H2O)(4)(-) cluster is confirmed using negative ion photoelectron spectroscopy, and the resulting spectrum suggests the presence of three isomeric forms for this species. (C) 2004 Elsevier B.V. All rights reserved.
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