Journal
CHEMICAL PHYSICS LETTERS
Volume 401, Issue 4-6, Pages 503-508Publisher
ELSEVIER
DOI: 10.1016/j.cplett.2004.09.156
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A novel perylene imide and oligo-pentaphenyl bisfluorene containing molecule is shown to undergo electron transfer to form an emissive charge transfer state in di-benzyl ether and THF. At the single molecule level in a PMMA film. fluorescence spectra characteristic of both emissive states (locally excited and charge transfer) are observed with 44% of the molecules studied showing switching between the two states. These results demonstrate that charge transfer fluorescence from single molecules can be used to report on the properties and dynamics of a molecule's immediate surroundings or nano-environment. (C) 2004 Elsevier B.V. All rights reserved.
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