Journal
ORGANIC LETTERS
Volume 7, Issue 3, Pages 479-482Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol047559e
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The first enantioselective total synthesis of tonantzitlolone, a novel 15-membered macrocyclic diterpene, utilized a Julia olefination, a highly selective, potassium enolate-based anti-Felkin aldol reaction, and an E-selective ring-closing metathesis as key C-C bond-forming steps. The absolute configuration of tonantzitlolone is established.
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