Journal
APPLIED ORGANOMETALLIC CHEMISTRY
Volume 28, Issue 3, Pages 198-203Publisher
WILEY
DOI: 10.1002/aoc.3109
Keywords
metal-organic framework; postsynthetic modification; copper iminopyridine complex; heterogeneous catalyst; 2-aminobenzothiazoles
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Funding
- National Natural Science Foundation of China [21172092, 20972057]
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A copper iminopyridine complex has been immobilized on to a metal-organic framework (MOF) through postsynthetic modification of IRMOF-3. The modified MOFs were fully demonstrated by using a variety of methods, and the structural integrity of the modified MOFs has been confirmed by powder X-ray diffraction (XRD). Furthermore, it was shown that the modified IRMOF-3 can act as an efficient solid catalyst for the synthesis of 2-aminobenzothiazoles via the reaction of 2-iodoanilines with isothiocyanates in a heterogeneous manner. Moreover, the catalyst could be facilely separated from the reaction mixture and reused for six consecutive cycles without significant degradation in catalytic activity. Copyright (c) 2014 John Wiley & Sons, Ltd.
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