Journal
PHYSICAL REVIEW LETTERS
Volume 94, Issue 8, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.94.083005
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It is shown that large nuclear polarizations in isolated molecules may be created via the hyperfine interaction following excitation to selected rotational states \JM>. Explicit time-dependent nuclear polarization expressions for pulsed rotational excitation are presented for the case of one nuclear spin I, and for the case of two nuclear spins I-1 and I-2 in the hierarchical coupling limit. Photodissociation of the polarized molecules allows the production of polarized atoms, on short time scales if pulsed, at densities close to the parent molecule density.
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