Journal
ORGANIC LETTERS
Volume 7, Issue 6, Pages 1047-1050Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol0473391
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A Bronsted acid-catalyzed highly stereoselective arene-ynamide cyclization is described. These reactions constitute a keteniminium variant of Pictet-Spengler cyclizations, leading to efficient synthesis of nitrogen heterocycles and related alkaloids. Total syntheses of desbromoarborescidines A and C are illustrated here as first applications of this methodology.
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