Journal
ORGANIC LETTERS
Volume 7, Issue 7, Pages 1255-1258Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol047331r
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- NIGMS NIH HHS [GM-47480] Funding Source: Medline
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Peptide-based chiral ligands, readily prepared from commercially available materials, are used to promote Cu-catalyzed asymmetric allylic alkylations of alpha,beta-unsaturated esters bearing a gamma-phosphate with various alkylzinc reagents. These transformations lead to the formation of alpha,alpha'-dialkyl-beta,gamma-unsaturated esters in high yields as well as high regio- (re) and enantioselectivities (ee).
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