Journal
CATALYSIS COMMUNICATIONS
Volume 6, Issue 4, Pages 301-305Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.catcom.2005.01.004
Keywords
N2O decomposition; zeolite; FER; BEA; ZSM5; ion-exchange; Fe zeolite catalysts
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This communication reports on the excellent performance and durability of a wet ion-exchanged Fe-Ferrierite catalysts for N2O decomposition under conditions of nitric acid plants, especially in the presence of water (0.5% vol) and at a high space time W/F-0(N2O) = 900 kg(cat) s mol(-1). In contrast to ion-exchange Fe-MFI catalysts, where a considerable deactivation is usually observed, iron species in the FER matrix seem to be much more stable in the presence of water, maintaining a high activity for more than 50 h on stream. (c) 2005 Elsevier B.V. All rights reserved.
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