4.8 Article

Efficient and long-lived field-free orientation of molecules by a single hybrid short pulse -: art. no. 153003

Journal

PHYSICAL REVIEW LETTERS
Volume 94, Issue 15, Pages -

Publisher

AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.94.153003

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We show that a combination of a half-cycle pulse and a short nonresonant laser pulse produces a strongly enhanced postpulse orientation. Robust transients that display both efficient and long-lived orientation are obtained. The mechanism is analyzed in terms of optimal oriented target states in finite Hilbert subspaces and shows that hybrid pulses can prove useful for other control issues.

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