4.8 Article

Time-dependent density functional theory of classical fluids

Journal

PHYSICAL REVIEW LETTERS
Volume 94, Issue 18, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.94.183001

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We establish a rigorous time-dependent density functional theory of classical fluids for a wide class of microscopic dynamics. We obtain a stationary action principle for the density. We further introduce an exact practical scheme, to obtain hydrodynamical effects in density evolution, that is analogous to the Kohn-Sham theory of quantum systems. Finally, we show how the current theory recovers existing phenomenological theories in an adiabatic limit.

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