Journal
MOLECULAR PHYSICS
Volume 103, Issue 13, Pages 1821-1827Publisher
TAYLOR & FRANCIS LTD
DOI: 10.1080/00268970500096103
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Preliminary findings are reported following the detailed analysis of intramolecular vibrational energy redistribution (IVR) in S-1 para-fluorotoluene following the excitation of one quantum in the CF stretching mode nu(7). It is shown that the method proposed has the potential to enable not only the determination of a rate constant for IVR, but also the identification of the dark states into which energy has redistributed. In addition energy flow has been observed from a bright state (11(+)) previously thought to be below the onset for IVR in this molecule, and evidence of mode-specificity in the IVR process.
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