Journal
JOURNAL OF PHYSICAL CHEMISTRY B
Volume 109, Issue 31, Pages 15093-15097Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jp052279h
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Thermodynamics and kinetics are thought to be linked in glass transitions. The quantitative predictions of alpha-relaxation activation barriers provided by the theory of glasses based on random first-order transitions are compared with the experimental results for 44 substances. The agreement found between the predicted activation energies near T-g and experiment is excellent. These predictions depend on the configurational heat capacity change on vitrification and the entropy of melting the crystal which are experimental inputs.
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