Journal
ORGANIC LETTERS
Volume 7, Issue 17, Pages 3781-3783Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol0515964
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The first enantioselective Bronsted acid catalyzed reduction of imines has been developed. This new organocatalytic transfer hydrogenation of ketimines with Hantzsch dihydropyridine as the hydrogen source offers a mild method to various chiral amines with high enantioselectivity. The stereochemistry of the chiral amines can be rationalized by a stereochemical model derived from an X-ray crystal structure of a chiral BINOL phosphate catalyst.
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