Journal
LANGMUIR
Volume 21, Issue 18, Pages 8333-8337Publisher
AMER CHEMICAL SOC
DOI: 10.1021/la050645i
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The decomposition of 1,1-dichloroethene on Pd(111) is investigated using conventional thermal desorption, laser-induced thermal desorption (LITD), and FT reflection absorption infrared spectroscopy (FT-RAIRS). The decomposition mechanism produces at least three hydrocarbon surface intermediates, including ethylidyne. Thermal desorption results differ between high and low coverages because of relative surface concentrations of Cl and H in combination with kinetic effects.
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