Journal
PHYSICAL REVIEW B
Volume 72, Issue 10, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.72.104402
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The Haldane system PbNi2V2O8 was investigated by temperature-dependent magnetization M(T) measurements at fields higher than H-c; H-c is the critical field required to close the Haldane gap. It has been revealed that for H > H-c, M(T) exhibits a cusplike minimum at T-min, below which it increases with a decrease in T following a convex curve. These results were observed for both H parallel to c and H perpendicular to c, with the c axis parallel to the chain. These data indicate the occurrence of field-induced magnetic ordering around T-min. The phase boundaries for H parallel to c and H perpendicular to c do not cross each other. This result is consistent with the theoretical calculation for a negative single-ion anisotropy D.
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