Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 11, Issue 24, Pages 7146-7153Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200500253
Keywords
cooperative effects; homogeneous catalysis; hydrogen bonds; P ligands; proton transfer
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Inspired by the cooperativity displayed by metalloenzymes, bifunctional organometallic complexes featuring pendant basic functional groups are designed and evaluated as catalysts in reactions for which enzymes are not suited. Anti-Markovnikov hydration of terminal alkynes is the focus, as are hydrogen bonding and proton transfer facilitated by the pendant groups.
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