Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 12, Issue 6, Pages 1715-1722Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200501038
Keywords
acidity; dynamic combinatorial chemistry; imines; molecular diversity; stimuli-responsive systems
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The constitutional recomposition of a dynamic library of imines displays a complex behavior under the effect of two parameters, acidity and temperature. A qualitative analysis of the quantitative data is presented. The results illustrate the response of such a dynamic system to a physical stimulus (temperature) and a chemical effector (H+), thus demonstrating its adaptive behavior under the pressure of external factors. They also point to the possibility of modulating a given functional property (optical, electronic, ionic) by constitutional recomposition induced by a specific trigger. Such features are of great interest for the development of stimuli-responsive, functional dynamic materials.
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