Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 71, Issue 6, Pages 2524-2527Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo052488y
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[GRAPHICS] In the presence of the Trost ligands-Pd catalysts, N-monoallylation of bis(2,4,6-triisopropylbenzne)sulfonylamides derived from mesa-1,2-diamines proceeds with good to excellent enantioselectivity (85-96% ee) to give asymmetric desymmetrization products. Under the same conditions, in the reaction with meso-bistolunesulfonylamide derivatives, reversal of the enantioselectivity is observed.
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