Journal
APPLIED PHYSICS LETTERS
Volume 88, Issue 14, Pages -Publisher
AMER INST PHYSICS
DOI: 10.1063/1.2192623
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Formation energies of possible vacancies under different oxygen partial pressures were studied using an ab initio density functional theory and supercell approach. Under oxygen-rich conditions, lead vacancies are the stable ones throughout the band gap, and their ionization level locates at 0.56 eV from the top of valence band, which may contribute to p-type conduction. Under oxygen-poor conditions, oxygen vacancies are the stable ones at the top of the valence band. It is a deep donor that may not only dilute the acceptor carriers to weaken the p-type conduction but hardly contribute to n-type conduction. (c) 2006 American Institute of Physics.
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