Journal
OPTICS LETTERS
Volume 31, Issue 10, Pages 1543-1545Publisher
OPTICAL SOC AMER
DOI: 10.1364/OL.31.001543
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- NIBIB NIH HHS [1 R01 EB001777] Funding Source: Medline
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To achieve high-spectral-resolution multiplex coherent anti-Stokes Raman scattering (CARS), one typically uses a narrowband pump pulse and a broadband Stokes pulse. This is to ensure a correspondence between anti-Stokes and vibrational frequencies. We obtain high-resolution CARS spectra of isopropanol, using a broadband chirped pump pulse and a broadband Stokes pulse, by detecting the anti-Stokes pulse with spectral interferometry. With the temporally resolved anti-Stokes signal, we can remove the chirp of the anti-Stokes pulse and restore high spectral resolution while also rejecting nonresonant scattering. (c) 2006 Optical Society of America.
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