Journal
CHEMICAL PHYSICS
Volume 324, Issue 2-3, Pages 398-404Publisher
ELSEVIER
DOI: 10.1016/j.chemphys.2005.11.005
Keywords
protonated tryptamine; protonated tryptophane; ab initio; excited states; photodissociation
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In very recent experiments, the excited-state lifetimes of protonated aromatic amino acids have been recorded by means of the pump-probe photodissociation technique. The excited-state decays are fast (picosecond time scale), leading to an extensive fragmentation of the protonated species. The calculations presented here for protonated tryptamine and tryptophan using a coupled-cluster method are meant to unravel the complex behavior of these systems. (c) 2005 Elsevier B.V. All rights reserved.
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