Journal
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
Volume 8, Issue 29, Pages 3440-3445Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/b607350f
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High resolution time-of-flight (TOF) measurements of the D atom fragments arising in the near ultraviolet (UV) photodissociation of deuterated pyrrole are reported. Structures evident in the measured TOF spectra are all interpretable in terms of N-D bond fission, and population of selected vibrational states of the pyrrolyl-d(4) co-fragment-thereby clarifying previous uncertainties regarding the branching into different vibronic states of the pyrrolyl radical following UV excitation of pyrrole.
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