4.6 Article

Diameter and chirality dependence of exciton properties in carbon nanotubes

Journal

PHYSICAL REVIEW B
Volume 74, Issue 12, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.74.121401

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We calculate the diameter and chirality dependences of the binding energies, sizes, and bright-dark splittings of excitons in semiconducting single-wall carbon nanotubes. Using results and insights from ab initio calculations, we employ a symmetry-based variational method within the effective-mass and envelope-function approximations using tight-binding wave functions. Binding energies and spatial extents show a leading dependence on diameter as 1/d and d, respectively, with chirality corrections providing a spread of roughly 20% with a strong family behavior. Bright-dark exciton splittings show a 1/d(2) leading dependence. We provide analytical expressions for the binding energies, sizes, and splittings that should be useful to guide future experiments.

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