Journal
TETRAHEDRON-ASYMMETRY
Volume 17, Issue 20, Pages 2847-2856Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetasy.2006.10.040
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Diastereomeric monosubstituted [2.2]paracyclophane-based N,O-ligands, which unite the planar and central chiral elements, were optimized for the enantio selective diethylzinc addition to aldehydes. (S)-1-{(S-p)-[2.2]Paracyclophan-4-yl} methyl-2-pyrrolidine-alpha,alpha-diphenylmethanol (S-p,S)-3 catalyzed the addition to give (R)-1-phenyl-l-propanol in a high yield and with a good enantio selectivity (91% ee). (c) 2006 Elsevier Ltd. All rights reserved.
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