Journal
TETRAHEDRON LETTERS
Volume 47, Issue 47, Pages 8423-8425Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tetlet.2006.09.040
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Radical reaction of a series of N-(2-bromoallyl)arylearboxamides led to the production of 4-arylpyrrolidin-2-ones and directly reduced materials in comparable yields. A cascade process, involving sequential 5-exo-trig spirocyclisation, beta-scission, and 5-endo-trig cyclisation of the resulting acyl radical, is proposed to explain the pyrrolidinone products. (c) 2006 Elsevier Ltd. All rights reserved.
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