Journal
JOURNAL OF PORPHYRINS AND PHTHALOCYANINES
Volume 11, Issue 3-4, Pages 151-159Publisher
WORLD SCI PUBL CO INC
DOI: 10.1142/S1088424607000199
Keywords
cation; anion; self-assembly; phthalocyanine; porphyrin; porphyrazine; electrochemistry; surface electrochemistry
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Self-assembled ion pairs are deposited onto a graphite electrode surface by dipping the electrode sequentially into phthalocyanine cations and anions, or a phthalocyanine cation and porphyrin anion. The electrochemical properties of these surface-bound ion pairs are compared with the properties of the individual surface-bound components. The order of deposition is shown to be crucial, implying that these species lie flat on the surface. A detailed study of the electrocatalytic oxidation of oxalate anion is used to explore their reactivity as a function of deposition order. Copyright (c) 2007 Society of Porphyrins & Phthalocyanines.
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