Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 57, Issue 35, Pages 11238-11241Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201805079
Keywords
alkanes; C-H activation; electrochemistry; oxidation; photocatalysis
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Funding
- International Joint Research Programs for Innovative Energy Technology
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The photo-electrochemical C-H bond activation of cyclohexane to produce cyclohexanol and cyclohexanone (KA oil) with high partial oxidation selectivity (99%) and high current utilization ratio (76%) was achieved in air at room temperature at atmospheric pressure. The production rate of KA oil was accelerated by applying a bias. The incident photon to current efficiencies at 365 and 420nm were 57% and 24%, respectively.
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