Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 57, Issue 39, Pages 12799-12803Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201807775
Keywords
asymmetric catalysis; boron; cross coupling; quaternary centers
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Funding
- NIH [R35-GM1217140]
- NATIONAL INSTITUTE OF GENERAL MEDICAL SCIENCES [R35GM127140] Funding Source: NIH RePORTER
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Catalytic enantioselective conjunctive cross-coupling has been developed to construct tertiary alkylboronic esters. These reactions occur with good yield and enantioselectivity for a range of substrates. Mechanistic experiments reveal aspects of the catalytic cycle that allow hindered substrates to react without significant complicating side reactions.
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