Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 57, Issue 44, Pages 14613-14618Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201807463
Keywords
CO2 activation; heterogeneous catalysis; methane dry reforming; photoelectron spectroscopy; X-ray diffraction
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Funding
- Austrian Science Fund [F4503-N16]
- EU Framework Programme for Research and Innovation HORIZON 2020 [730872]
- DOE Office of Science User Facility [DE-AC02-05CH11231]
- ALS doctoral fellowship
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C-saturated Pd-0 nanoparticles with an extended phase boundary to ZrO2 evolve from a (PdZr0)-Zr-0 precatalyst under CH4 dry reforming conditions. This highly active catalyst state fosters bifunctional action: CO2 is efficiently activated at oxidic phase boundary sites and PdxC provides fast supply of C-atoms toward the latter.
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