Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 53, Issue 8, Pages 2152-2156Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201308354
Keywords
electrochemistry; energy storage; layered compounds; molybdenum; nanostructures
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Funding
- Alexander von Humboldt Foundation (Sofja Kovalevskaja award)
- National Natural Science Foundation of China [21171015, 21373195]
- Chinese Government
- Fundamental Research Funds for the Central Universities [WK2060140014]
- Max Planck Society
- European Union [312483 (ESTEEM2)]
- program for New Century Excellent Talents in University (NCET)
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The preparation and electrochemical storage behavior of MoS2 nanodotsmore precisely single-layered ultrasmall nanoplatesembedded in carbon nanowires has been studied. The preparation is achieved by an electrospinning process that can be easily scaled up. The rate performance and cycling stability of both lithium and sodium storage were found to be outstanding. The storage behavior is, moreover, highly exciting from a fundamental point of view, as the differences between the usual storage modesinsertion, conversion, interfacial storageare beneficially blurred. The restriction to ultrasmall reaction domains allows for an almost diffusion-less and nucleation-free conversion, thereby resulting in a high capacity and a remarkable cycling performance.
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