Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 53, Issue 50, Pages 13840-13844Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201406626
Keywords
hapalindole; indole terpenoids; Prins cyclization
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Funding
- Ministry of Science Technology [2013CB836900]
- National Natural Science Foundation of China [21290180, 21172235, 21222202]
- Pujiang Program [12J1410800]
- China Postdoctoral Science Foundation [2014M551480]
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A unified and bioinspired oxidative cyclization strategy was used in the first total syntheses of naturally occurring 12-epi-hapalindoleQ isonitrile, hapalonamideH, deschloro 12-epi-fischerindoleI nitrile, and deschloro 12-epi-fischerindoleW nitrile, as well as the structural revision of the latter. HapalindolesH and Q were also synthesized.
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