Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 53, Issue 18, Pages 4603-4607Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201310438
Keywords
fluorescence; intramolecular charge transfer; photochromism; quantum yield; steric hindrance
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Funding
- National 973 Program [2013CB733700]
- NSFC/China
- NSFC for Distinguished Young Scholars [21325625]
- Oriental Scholarship
- National Major Scientific Technological Special Project [2012YQ15008709]
- SRFDP [20120074110002]
- Fundamental Research Funds for the Central Universities [WK1013002]
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Endowing both solvent independency and excellent thermal bistability, the benzobis(thiadiazole)-bridged diarylethene system provides an efficient approach to realize extremely high photocyclization quantum yields (phi(o-c), up to 90.6%) by both separating completely pure anti-parallel conformer and suppressing intramolecular charge transfer (ICT).
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