Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 53, Issue 13, Pages 3505-3509Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201308601
Keywords
axial chirality; C-H activation; dehydrogenative cross-couplings; lauternamines; oxidative amination
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Funding
- DFG [SFB/TRR 88]
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The dehydrogenative C-N cross-coupling of unprotected, secondary anilines through ortho-N-carbazolation has been achieved using a Ru catalytic system with O-2 as the terminal oxidant. The reactions proceed in an intermolecular fashion, selectively in the ortho position. Implications for the field of organic synthesis are discussed.
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