Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 53, Issue 23, Pages 5852-5857Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201310461
Keywords
artificial photosynthesis; photocathodes; photoelectrochemical CO2 reduction; solution synthesis; zinc telluride
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Funding
- BK+ Program
- Basic Science Research Program [2012-017247]
- Korea Center for Artificial Photosynthesis (KCAP) - National Research Foundation of Korea [2012M1A2A2671779]
- National Research Foundation of Korea [2012M1A2A2671779] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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As a photocathode for CO2 reduction, zinc-blende zinc telluride (ZnTe) was directly formed on a Zn/ZnO nanowire substrate by a simple dissolution-recrystallization mechanism without any surfactant. With the most negative conduction-band edge among p-type semiconductors, this new photocatalyst showed efficient and stable CO formation in photoelectrochemical CO2 reduction at -0.2--0.7 V versus RHE without a sacrificial reagent.
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