Journal
PHYSICAL REVIEW LETTERS
Volume 98, Issue 7, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.98.073003
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Using H-2(+) and D-2(+), we observe two-surface population dynamics by me(+) (D-2(+)) ionize in short (40-140 fs) and intense (10(14) W/cm(2)) infrared laser pulses. Experimentally, we find a modulation of the kinetic energy spectrum of the correlated fragments. The spectral progression arises from a hitherto unexpected spatial modulation on the excited state population, revealed by Coulomb explosion. By solving the two-level time-dependent Schrodinger equation, we show that an interference between the net-two-photon and the one-photon transition creates localized electrons which subsequently ionize.
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