Journal
SOLID STATE COMMUNICATIONS
Volume 141, Issue 11, Pages 587-590Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ssc.2007.01.009
Keywords
(BaxSr1-x)(0.77)Ca0.23TiO3; ceramic; ferroelectric properties; polarization
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The dielectric and ferroelectric properties of (BaxSr1-x)(0.77)Ca0.23TiO3 ceramics with x = 1 to 0.7 were studied and compared with those of BaxSr1-xTiO3 and Ba0.77Ca0.23TiO3 ceramics. It has been found that Sr doping of the Ba0.77Ca0.23TiO3 ceramics causes a drastic decrease of the Curie temperature, just like Sr doping of pure BaTiO3 ceramics, demonstrating a cell volume effect. However, the (BaxSr1-x)(0.77)Ca0.23TiO3 ceramics with x = 0.9 and 0.8 have larger spontaneous polarization than those of the corresponding BaxSr1-xTiO3 and Ba0.77Ca0.23TiO3 ceramics, along with sufficient insulating properties. The enhancement of their polarization was explained by the increase of the lattice parameter c/a ratio due to the lattice distortion and strain developed in the ceramics. (C) 2007 Elsevier Ltd. All rights reserved.
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