Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 53, Issue 1, Pages 74-100Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.201304268
Keywords
CC coupling; C-H activation; cross-coupling; green chemistry; synthetic methods
Categories
Funding
- DAAD (German Academic Exchange Service)
- McGill University
- NSERC
- FQRNT
- CFI
- E. B. Eddy Endowment Fund
- Canada Research Chair
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Over the last decade, substantial research has led to the introduction of an impressive number of efficient procedures which allow the selective construction of CC bonds by directly connecting two different CH bonds under oxidative conditions. Common to these methodologies is the generation of the reactive intermediates in situ by activation of both CH bonds. This strategy was introduced by the group of Li as cross-dehydrogenative coupling (CDC) and discloses waste-minimized synthetic alternatives to classic coupling procedures which rely on the use of prefunctionalized starting materials. This Review highlights the recent progress in the field of cross-dehydrogenative Csp3C formations and provides a comprehensive overview on existing procedures and employed methodologies.
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