4.8 Article

Magnetothermal transport in the spin-1/2 chains of copper pyrazine dinitrate

Journal

PHYSICAL REVIEW LETTERS
Volume 98, Issue 10, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.98.107201

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We present experiments on the thermal transport in the spin-1/2 chain compound copper pyrazine dinitrate Cu(C4H4N2)(NO3)(2). The heat conductivity shows a surprisingly strong dependence on the applied magnetic field B, characterized at low temperatures by two main features. The first one appearing at low B is a characteristic dip located at mu B-B similar to k(B)T, that may arise from umklapp scattering. The second one is a plateaulike feature in the quantum critical regime, mu(B)vertical bar B-B-c vertical bar < k(B)T, where B-c is the saturation field at T=0. The latter feature clearly points towards a momentum and field-independent mean free path of the spin excitations, contrary to theoretical expectations.

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