4.8 Article

Ex situ aqueous mineral carbonation

Journal

ENVIRONMENTAL SCIENCE & TECHNOLOGY
Volume 41, Issue 7, Pages 2587-2593

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/es0619253

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The U.S. Department of Energy's National Energy Technology Laboratory (NETL) located in Albany, OR (formerly the Albany Research Center) has studied ex situ mineral carbonation as a potential option for carbon dioxide sequestration. Studies focused on the reaction of Ca-, Fe-, and Mg-silicate minerals with gaseous CO2 to form geologically stable, naturally occurring solid carbonate minerals. The research included resource evaluation, kinetic studies, process development, and economic evaluation. An initial cost estimate of similar to$69/ton of CO2 sequestered was improved with process improvements to similar to$54/ton. The scale of ex situ mineral carbonation operations, requiring similar to 55 000 tons of mineral to carbonate, the daily CO2 emissions from a 1-GW, coal-fired power plant, may make such operations impractical.

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