Journal
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY
Volume 32, Issue 7, Pages 796-801Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.ijhydene.2006.12.012
Keywords
solid oxide fuel cell; direct alcohol fuelling; cathode materials; methanol ethanol; ceria composite electrolyte
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We have made extensive efforts to develop various compatible cathode materials for the ceria-carbonate composite (CCC) electrolytes to be used in direct alcohol fuelled solid oxide fuel cells (DLFC). The following cathode materials were mainly investigated: (i) BSCF (BaSrCoFeO) perovskite oxide; (ii) LFN (LaFeO-based oxides, e.g. LaFe0.8Ni0.2O3) perovskite oxides; (iii) bi- or tri-phase metal oxides with or without lithiation. A number of copper- and nickel-based anode composites were also developed for methanol and ethanol with maximum catalytic activity. The tri-metal oxide (CuNiOx-ZnO) cathode produced the maximum power density output of 500 mW/cm(-2) at 580 degrees C for DLFC with methanol operation. (c) 2007 International Association for Hydrogen Energy. Published by Elsevier Ltd. All rights reserved.
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