Journal
ORGANIC LETTERS
Volume 9, Issue 10, Pages 1967-1970Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol0705548
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Second-generation ruthenium carbenoid catalysts for olefin metathesis are a hundred to a thousand times more active than first-generation catalysts, despite a slower initiation step. A new density functional capable of treating medium-range correlation energy shows that the relative rates of generation of the catalyst are determined by attractive noncovalent interactions.
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