4.8 Article

Magnetic susceptibility of the Kagome antiferromagnet ZnCu3(OH)6Cl2

Journal

PHYSICAL REVIEW LETTERS
Volume 98, Issue 20, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.98.207204

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We analyze the experimental data for the magnetic susceptibility of the material ZnCu3(OH)(6)Cl-2 in terms of the Kagome Lattice Heisenberg model (KLHM), discussing possible role of impurity spins, dilution, exchange anisotropy, and both out-of-plane and in-plane Dzyloshinski-Moriya (DM) anisotropies, with explicit theoretical calculations using the numerical linked cluster method and exact diagonalization. The high-temperature experimental data are well described by the pure Heisenberg model with J=170 K. We show that the sudden upturn in the susceptibility around T=75 K is due to DM interactions. We also observe that at intermediate temperatures, below T=J, our calculated susceptibility for KLHM fits well with a power law T-0.25.

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