Journal
PHYSICAL REVIEW LETTERS
Volume 98, Issue 21, Pages -Publisher
AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.98.216601
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An experimental demonstration of electrical detection of coherent spin motion of weakly coupled, localized electron spins in thin fullerene C-60 films at room temperature is presented. Pulsed electrically detected magnetic resonance experiments on vertical photocurrents through Al/C-60/ZnO samples showed that an electron spin Rabi oscillation is reflected by transient current changes. The nature of possible microscopic mechanisms responsible for this spin to charge conversion as well as its implications for the readout of endohedral fullerene (N@C-60) spin qubits are discussed.
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