Journal
PHYSICAL REVIEW LETTERS
Volume 98, Issue 22, Pages -Publisher
AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.98.220501
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Funding
- EPSRC [EP/D048559/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/D048559/1] Funding Source: researchfish
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By applying a new technique for dynamic nuclear polarization involving simultaneous excitation of electronic and nuclear transitions, we have enhanced the nuclear polarization of the nitrogen nuclei in N-15@C-60 by a factor of 10(3) at a fixed temperature of 3 K and a magnetic field of 8.6 T, more than twice the maximum enhancement reported to date. This methodology will allow the initialization of the nuclear qubit in schemes exploiting N@C-60 molecules as components of a quantum information processing device.
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