Journal
CHEMPHYSCHEM
Volume 8, Issue 8, Pages 1215-1220Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cphc.200700091
Keywords
fluorescence; host-guest systems; laser spectroscopy; molecular electronics; single-molecule studies
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We study, single dibenzoterrylene molecules in an anthrocene single crystal at 1.4 K in two insertion sites at 785.1 and 794.3 nm. The single-molecule zero-phonon lines are, narrow (about 30 MHz), intense (the detected fluorescence rates at saturation reach 100,000 counts s(-1)), and very photostable. The intersystem-crossing yield is extremely low (10(-7) or lower). All of these features are hallmarks of an excellent system for high-resolution spectroscopy and nonoscale probing at cryogenic temperatures.
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