Journal
ORGANIC LETTERS
Volume 9, Issue 12, Pages 2253-2256Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol070263z
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A very simple annulation reaction was designed, allowing an imidazole moiety to be fused onto a range of pyridine-based derivatives. The methodology consists of an activation step via the formation of a pyridinium salt to increase the electrophilicity of the pyridine ring, followed by a cascade reaction triggered by a nucleophilic attack of the iminium moiety. Depending on the pyridinium salt, it is possible to obtain functionalized imidazole moieties.
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